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EU-wide monitoring survey on emerging polar organic contaminants in wastewater treatment plant effluents

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LOOS Robert CARVALHO Raquel ANTONIO Diana C CORNERO Sara LOCORO Giovanni TAVAZZI Simona PARACCHINI Bruno GHIANI Michela LETTIERI Teresa BLÁHA Luděk JAROŠOVÁ Barbora VOORSPOELS Stefan SERVAES Kelly HAGLUND Peter FICK Jerker LINDBERG Richard H SCHWESIG David GAWLIK Bernd M

Rok publikování 2013
Druh Článek v odborném periodiku
Časopis / Zdroj Water Research
Fakulta / Pracoviště MU

Přírodovědecká fakulta

Citace
Doi http://dx.doi.org/10.1016/j.watres.2013.08.024
Obor Znečištění a kontrola vody
Klíčová slova Wastewater treatment plants (WWTPs); Effluent water; European wide monitoring; Polar organic contaminants; Pharmaceuticals and personal care products (PPCPs)
Popis In the year 2010, effluents from 90 European wastewater treatment plants (WWTPs) were analyzed for 156 polar organic chemical contaminants. The analyses were complemented by effect-based monitoring approaches aiming at estrogenicity and dioxin-like toxicity analyzed by in vitro reporter gene bioassays, and yeast and diatom culture acute toxicity optical bioassays. Analyses of organic substances were performed by SPE or LLE followed by LC-MS-MS or GC-HRMS. Target microcontaminants were pharmaceuticals and personal care products (PPCPs), veterinary drugs, perfluoroalkyl substances (PFASs), organophosphate ester flame retardants, pesticides (and some metabolites), industrial chemicals such as benzotriazoles (corrosion inhibitors), iodinated x-ray contrast agents, and gadolinium magnetic resonance imaging agents; in addition biological endpoints were measured. The obtained results show the presence of 125 substances (80% of the target compounds) in European wastewater effluents, in concentrations ranging from low nanograms to milligrams per liter. These results allow for an estimation to be made of a European median level for the chemicals investigated in WWTP effluents. The most relevant compounds in the effluent waters with the highest median concentration levels were the artificial sweeteners acesulfame and sucralose, benzotriazoles (corrosion inhibitors), several organophosphate ester flame retardants and plasticizers (e.g. tris(2-chloroisopropyl)phosphate; TCPP), pharmaceutical compounds such as carbamazepine, tramadol, telmisartan, venlafaxine, irbesartan, fluconazole, oxazepam, fexofenadine, diclofenac, citalopram, codeine, bisoprolol, eprosartan, the antibiotics trimethoprim, ciprofloxacine, sulfamethoxazole, and clindamycine, the insect repellent N,N'-diethyltoluamide (DEET), the pesticides MCPA and mecoprop, perfluoroalkyl substances (such as PFOS and PFOA), caffeine, and gadolinium.
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