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Temperature Dependence of Relativistic Valence Band Splitting Induced by an Altermagnetic Phase Transition

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HAJLAOUI Mahdi D'SOUZA Sunil Wilfred ŠMEJKAL Libor KRIEGNER Dominik KRIZMAN Gauthier ZAKUSYLO Tetiana OLSZOWSKA Natalia CAHA Ondřej MICHALIČKA Jan SANCHEZ-BARRIGA Jaime MARMODORO Alberto VÝBORNÝ Karel ERNST Arthur CINCHETTI Mirko MINAR Jan JUNGWIRTH Tomas SPRINGHOLZ Gunther

Rok publikování 2024
Druh Článek v odborném periodiku
Časopis / Zdroj Advanced Materials
Fakulta / Pracoviště MU

Přírodovědecká fakulta

Citace
www https://onlinelibrary.wiley.com/doi/full/10.1002/adma.202314076
Doi http://dx.doi.org/10.1002/adma.202314076
Klíčová slova altermagnetism; angle-resolved photoemission spectroscopy; electronic band structure; spintronics
Popis Altermagnetic (AM) materials exhibit non-relativistic, momentum-dependent spin-split states, ushering in new opportunities for spin electronic devices. While the characteristics of spin-splitting are documented within the framework of the non-relativistic spin group symmetry, there is limited exploration of the inclusion of relativistic symmetry and its impact on the emergence of a novel spin-splitting in the band structure. This study delves into the intricate relativistic electronic structure of an AM material, alpha-MnTe. Employing temperature-dependent angle-resolved photoelectron spectroscopy across the AM phase transition, the emergence of a relativistic valence band splitting concurrent with the establishment of magnetic order is elucidated. This discovery is validated through disordered local moment calculations, modeling the influence of magnetic order on the electronic structure and confirming the magnetic origin of the observed splitting. The temperature-dependent splitting is ascribed to the advent of relativistic spin-splitting resulting from the strengthening of AM order in alpha-MnTe as the temperature decreases. This sheds light on a previously unexplored facet of this intriguing material.

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